光催化还原二氧化碳制备太阳燃料研究进展及挑战
发布时间：2018-10-30 20:14
【摘要】：光催化还原二氧化碳制备太阳燃料是太阳能转化与利用的主要发展方向之一,其核心是构建高效的光催化反应体系.本文介绍光催化还原二氧化碳反应的基本原理与改善能量转化效率的主要途径,综述了微结构设计、晶体工程、电子结构设计等改善光催化材料催化活性的方法,探讨光催化反应中的基本物理化学问题以及高效光催化材料开发的主要策略.分析了影响能量转换效率的关键因素及开展光催化反应热力学与动力学研究的重要性,评述了几种新型光化学还原CO_2的反应,展望了该领域的未来发展方向.
[Abstract]:Photocatalytic reduction of carbon dioxide to prepare solar fuel is one of the main development directions of solar energy conversion and utilization, the core of which is to construct an efficient photocatalytic reaction system. In this paper, the basic principle of photocatalytic reduction of carbon dioxide and the main ways to improve the efficiency of energy conversion are introduced. The methods of improving the catalytic activity of photocatalytic materials such as microstructure design, crystal engineering and electronic structure design are reviewed. The basic physical and chemical problems in photocatalytic reactions and the main strategies for the development of highly efficient photocatalytic materials are discussed. The key factors affecting energy conversion efficiency and the importance of studying thermodynamics and kinetics of photocatalytic reaction are analyzed. Several new photochemical reduction CO_2 reactions are reviewed and the future development of this field is prospected.
【作者单位】： 南京大学现代工程与应用科学学院环境材料与再生能源研究中心;
【基金】：国家重点基础研究发展计划(编号:2013CB632404) 国家自然科学基金(编号:51572121,21603098,2163300,11504162) 国民核生化灾害防护国家重点实验室开放课题(编号:SKLNBC2014-09) 江苏省自然科学基金(编号:BK20151265,BK20150580)资助项目
【分类号】：O643.3;O644.1
[Abstract]:Photocatalytic reduction of carbon dioxide to prepare solar fuel is one of the main development directions of solar energy conversion and utilization, the core of which is to construct an efficient photocatalytic reaction system. In this paper, the basic principle of photocatalytic reduction of carbon dioxide and the main ways to improve the efficiency of energy conversion are introduced. The methods of improving the catalytic activity of photocatalytic materials such as microstructure design, crystal engineering and electronic structure design are reviewed. The basic physical and chemical problems in photocatalytic reactions and the main strategies for the development of highly efficient photocatalytic materials are discussed. The key factors affecting energy conversion efficiency and the importance of studying thermodynamics and kinetics of photocatalytic reaction are analyzed. Several new photochemical reduction CO_2 reactions are reviewed and the future development of this field is prospected.
【作者单位】： 南京大学现代工程与应用科学学院环境材料与再生能源研究中心;
【基金】：国家重点基础研究发展计划(编号:2013CB632404) 国家自然科学基金(编号:51572121,21603098,2163300,11504162) 国民核生化灾害防护国家重点实验室开放课题(编号:SKLNBC2014-09) 江苏省自然科学基金(编号:BK20151265,BK20150580)资助项目
【分类号】：O643.3;O644.1
【相似文献】
相关期刊论文 前10条
1 赵毅;刘威;张自丽;祝晓雨;;光催化还原二氧化碳影响因素分析[J];中国电力;2013年01期
2 史载锋,张苏敏,林小明;光催化还原法制备载银二氧化钛[J];海南师范学院学报(自然科学版);2001年04期
3 张昊,谭欣,赵林;废水中重金属离子的光催化还原研究进展[J];天津理工学院学报;2004年03期
4 张天永,由兰英,张友兰,赵进才;石英反应器中硝基物的光催化还原[J];精细化工;2005年03期
5 孙彦;陈亮;陈东辉;黄满红;;光催化还原十溴联苯醚[J];广州化工;2012年01期
6 付宏祥，吕功煊，，李新勇，李树本;重金属离子的光催化还原研究进展[J];感光科学与光化学;1995年04期
7 孟元华;;杂多酸光催化还原回收废水中银的试验探讨[J];职业与健康;2014年01期
8 徐玉欣,李越湘,彭绍琴;银铜离子复合体系的光催化还原[J];环境化学;2004年05期
9 缪应纯;王刚;高亚玲;吴仕鹏;;光催化还原硝酸根的研究进展[J];安徽农业科学;2012年34期
10 鞠春红;张伟君;王志成;李福
本文编号：2301058
本文链接：https://www.wllwen.com/kejilunwen/huaxue/2301058.html
教材专著
